Out-of-phase ESEEM pulse sequence with the first pulse set to pi/4 to probe two-electron correlations in the initial condition.
parameters.npoints number of time points to be computed parameters.timestep simulation time step, seconds parameters.rho0 initial state parameters.coil detection state parameters.screen optional screen state (must be the Hermitian conjugate of the detection state) parameters.pulse_op pulse operator A, the propagators for the pulses will be exp(-i*A*pi) and exp(-i*A*pi/4) H - Hamiltonian matrix, received from context function R - relaxation superoperator, received from context function K - kinetics superoperator, received from context function
fid - OOP-ESEEM time trace
Figure 3a in http://dx.doi.org/10.1021/bi048445d is reproduced in examples/esr_solids/oop_eseem_photosystem_1.m example file. The output appears below.
The sequence uses ideal pulses, replace with calls to shaped_pulse_af.m to have soft pulses instead.